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PRECISE MASSES AND ISOTOPE STUDIES1

Mass Spectrometers for Precise Mass Determinations＆H．MATSUDA3

Mass Differences of the Doublets Including C,H,D,and 35Cl and Preliminary Mass Values of H,D,and 35Cl＆ITSUO KATAKUSE,HIROMITSU NAKABUSHI,AND KOREICHI OGATA10

Mass Spectrometry and Measurement of Neutron Reaction Cross-sections for Power Nuclear Reactor Operation＆G．NIFE AND E．ROTH14

Mass Spectrometric Study of the Rate Production of the Light Elements (Li,Be,B) and Applications to Astrophysics＆R．BERNAS34

THEORY OF MASS SPECTRA41

Potential Energy Surfaces of Molecular Ions＆J．C．LORQUET,A．J．LORQUET,J．C．LECLERC,AND C．CADET43

A Ballistic Theory of Ion Breakdown＆P．F．KNEWSTUBB48

Statistical Rate Theory for Systems of Morse Oscillators and its Application to the Theory of Mass Spectra＆Z．PRASIL53

The Dynamic Theory of Field Ionization＆I．V．GOLDENFELD,E．N．KOROL,V．A．NAVARENKO,AND V．A．POKROVSKY58

Second Differential Ionization Efficiencies and the Ionization and Fragmentation of Olefins＆G．G．MEISELS AND B．G．GIESSNER61

Charge Separation and Ion Pair Formation in Cations＆J．SEIBL67

Monomolecular and Collision-Induced Pre-dissociation in the Mass Spectrum of N2＆J．MOMIGNY and H．WANKENNE70

IONIZATION PROCESSES79

The Ionization Process＆H．EHRHARDT81

New Results in the Field of Photo-ionization＆BURKHARD BREHM90

Angular Distributions of Photo-electrons＆R．MORGENSTERN,A．NIEHAUS,AND M．W．RUF100

The Photo-electron Spectra of some Small Molecules＆A．B．CORNFORD,D．C．FROST,C．A．MCDOWELL,J．L．RAGLE,AND A．I．STENHOUSE105

Photo-electron Spectra and Chemical Bonding of MercuryⅡCompounds＆J．H．D．ELAND108

Photo-ionization Studies of F2,HF,DF,and the Xenon Fluorides＆J．BERKOWITZ,W．A．CHUPKA,P．M．GUYON,J．HOLLOWAY,AND R．SPOHR112

Comparison of Penning-Ionization and Photo-ionization of Simple Molecules＆H．HOTOP116

A Pulsed Mass Spectrometric Study of Penning-Ionization in Helium-Argon Mixtures＆J．J．DECORPO AND F．W．LAMPE121

Mass and Phase Spectrometry of Heated SF6 and CO2＆R．T．BRACKMANN,W．L．FITE,AND W．M．JACKSON125

Neutral Fragment Mass Spectrometry＆K．O．DYSON128

Absolute Ionization Cross-section of Alkali Atoms by Electron Impact＆R．JALIN,R．HAGEMANN,P．LOHEZ,AND R．BOTTER133

A New Method of Studying Molecules by Electron Impact Spectroscopy＆F．W．E．KNOOP,H．H．BRONGERSMA,A．J．H．BOERBOOM,AND L．J．OOSTERHOFF136

ATOMIC AND MOLECULAR COLLISIONS141

Excitation in Collisions Between Ions and Atoms Observed by Light Intensity Measurements＆F．J．DE HEER143

Charge Exchange in Merging Beams＆F．BROUILLARD153

Energy Distribution in the Products of Ionic Reactions＆D．A．BAFUS,J．J．DECORPO,AND J．L．FRANKLIN159

Angular Distribution of H(2S) in Collision-Induced Dissociation of H+2＆D．H．JAECKS,D．H．CRANDALL,AND R．H．MCKNIGHT164

The Angular Dependence of the He+ dissociation Fragments of (HeH)+＆J．SCHOPMAN,J．LOS,AND J．MAAS168

Multiple Ionization of Ar by 10 keV Electrons as a Function of the Energy Loss＆M．J．VAN DER WIEL and F．J．DE HEER172

Fragmentation of Propane by Dissociative Charge Transfer．Studies by Translational Energy Ion Spectroscopy and by Time-resolved Ion Spectroscopy＆ROY S．LEHRLE,JOHN E．PARKER,AND JAMES C．ROBB174

Mass Spectrometric Study of Ionization and Fragmentation of Simple Molecular Gases by 5-45 keV Helium Atoms＆R．BROWNING,C．J．LATIMER,AND H．B．GILBODY179

Dissociation of Molecule-Ions Formed by Charge Exchange Collisions in an In-line Tandem Mass Spectrometer＆THOMAS O．TIERNAN AND CHAVA LIFSHITZ184

Reactions of Alkali Atoms with Atmosphere Ions＆P．K．ROL189

ION-MOLECULE REACTIONS193

Ion Cyclotron Resonance Mass Spectrometry＆GILLIAN C．GOODE,REBECCA M．O＇MALLEY,A．J．FERRER-CORREIA,AND K．R．JENNINGS195

Ion-Molecule Reactions of Small Molecules by Ion Cyclotron Resonance Mass Spectroscopy＆J．H．FUTRELL,D．SMITH,AND R．CLOW202

The Study of Ion-Neutral Collision Processes with a Pulsed Tandem Mass Spectrometer＆A．J．MASSON,P．F．FENNELLY,AND M．J．HENCHMAN207

Beam Studies of Several Elementary Ion Molecule Reactions＆J．KRENOS,P．HIERL,J．TULLY,Z．HERMAN,AND R．WOLFGANG213

Negative Ion-Neutral Molecule Interactions by Pulse Methods＆I．PLATZNER,G．LEVIN,AND F．S．KLEIN217

On the Reaction Mechanism of Some Negative Ion Molecule Reactions at Low Energies (Some eV-200 eV)＆D．VOGT222

Studies of Gaseous Ionic Equilibria in the Methane-Water and Propane-Water Systems＆F．H．FIELD AND D．P．BEGGS226

Clustering Reactions of the Hydronium Ion＆C．E．YOUNG,D．EDELSON,AND W．E．FALCONER229

Studies in Chemical Ionization Mass Spectrometry＆JOHN MICHNOWICZ AND BURNABY MUNSON233

Charge-Exchange Spectra of Some Substituted Benzophenones and N-Substituted Phenyl Benzamides＆ROBERT H．SHAPIRO AND JONATHAN TURK238

Photo-ionization-Induced Ion-Molecule Reactions in Nitric Oxide and Nitrogen Dioxide＆J．YINON AND F．S．KLEIN241

INSTRUMENTATION249

Selected Topics in Instrumentation－A Review＆RICHARD E．HONIG249

Application of Matrix Calculation in Ion Optics＆A．J．H．BOERBOOM269

The Spiratron＆J．M．B．BAKKER278

High-Intensity Mass Spectrometers＆S．B．KARMOHAPATRO283

Matsuda Type Virtual Image Double-Focusing Mass Spectrometer JMS-06＆M．ISHIBASHI,M．NOJIRI,AND E．WATANABE286

An Inhomogeneous Oscillatory Electric Field Time-of-Flight Mass Spectrometer＆J．P．CARRICO,L．D．FERGUSON,AND R．K．MUELLER292

Split-Screen Storage Oscilloscope for GLC/MS Peak Monitoring＆H．H．BOVEE AND L．E．MONTEITH295

Some New Ways of Studying Metastable Ion Decompositions＆R．M．CAPRIOLI,J．H．BEYNON,W．E．BAITINGER,AND J．W．AMY297

A New Method of Examining Metastable Ions Formed by Electron Impact Ionization of Organic Molecules＆N．R．DALY,A．MCCORMICK,AND R．E．POWELL300

DATA PROCESSING305

Progress of the Mass Spectrometry Data Centre,1966-70＆R．G．RIDLEY307

The Application of Artificial Intelligence in the Interpretation of Low-Resolution Mass Spectra＆ARMAND BUCHS,ALLAN B．DELFINO,CARL DJERASSI,A．M．DUFFIELD,B．G．BUCHANAN,E．A．FEIGENBAUM,J．LEDERBERG,GUSTAV SCHROLL,AND G．L．SUTHERLAND314

An Approach to Quantitative Mass Spectral Analysis＆THOMAS R．EDWARDS193

Automatic Evaluation of Photo-plates in Spark-Source Mass Spectrometry＆J．FRANZEN,W．SCHONFELD,AND D．STUWER322

On-line Data Acquisition and Interpretation of Spark-Source Mass Spectra＆R．A．BINGHAM,R．BROWN,AND P．POWERS326

Mass Spectrometric Data Acquisition and Handling－a Modular,Lowcost,High-Performance System＆A．CARRICK330

On-line Computer Methods Used in Conjunction with the Measurement of Ionization and Appearance Potentials＆R．A．W．JOHNSTONE,F．A．MELLON,AND S．D．WARD334

Data Processing of Isotopic Mass Spectra＆R．BIR339

Digital,Techniques in Connection with Isotopic Mass Spectrometry．1．Gas and Solid High Isotopic Ratios＆J．P．BOULLOUD,C．JONNET,J．MARAGNON,AND P．TAUVERON344

INOGRANIC AND HIGH-TEMPERATURE CHEMISTRY347

Mass Spectrometric Studies in High-Temperature Chemistry＆L．N．GOROKHOV AND G．A．SEMENOV349

The Determination of Thermodynamic Activities in High-Temperature Solutions by Mass Spectrometry＆G．R．BELTON359

The Use of a Highly Sensitive Mass Spectrometer for Thermodynamic and Phase Relationship Studies in Carbide Systems＆EDMUND STORMS369

High-Temperature Mass Spectrometric Studies of Some Rare-Earth-Carbon and Transition Metal-Carbon Systems＆CARL A．STEARNS AND FRED J．KOHL371

Thermodynamics of the Titanium Oxides＆PAUL W．GILLES AND PETER J．HAMPSON374

Mass Spectrometry of Anhydrous Metal Nitrate Vapours＆I．LAUDER,C．TOWLER,AND T．WUTH379

Thermodynamic Activities in the Ternary System Cr-Fe-Ni at 1600° C by Mass Spectrometry＆SIGURD WAGNER AND GEORGE R．ST．PIERRE388

Mass Spectrometric Investigation of Two-Component Systems of Complex Vapour Composition by the Isothermal Evaporation Method＆L．N．SIDOROV,V．I．BELOUSOV,AND V．B．SCHOLTZ394

Study of the Ionization Processes of Metal Vapours by Means of a Fox Source Coupled with a Knudsen Cell＆B．CABAUD,R．UZAN,AND P．NOUNOU399

Field Ion Mass Spectra of Selenium＆HORST SAURE AND JOCHEN BLOCK404

Relative Ionization Cross-sections of Transition Metals using Time-of-Flight Mass Spectrometry＆EDMUND J．ROLINSKI,CHARLES J．OBLINGER,AND MICHAEL HOCH408

Systematic Study of the Decomposition of Very Small Quantities of Lanthanide Oxides in the Presence of Heated Metallic Rhenium＆NGUYEN-LONG-DEN AND M．DE SAINT SIMON413

SECONDARY ION EMISSION AND SURFACE PHENOMENA417

Secondary Ion Emission from Solid Surfaces＆R．CASTAING AND J．-F．HENNEQUIN419

The Atom-Probe Field Ion Microscope＆ERWIN W．MULLER427

A Combined Ion and Electron Microprobe＆H．LIEBL433

Analytical Applications of an Ion Microprobe Mass Spectrometer-Negative Ion Spectroscopy＆CHARLES A．EVANS,Jr436

Analysis of Thin Films by Ion Microprobe Mass Analyser＆H．TAMURA,T．KONDO,AND H．DOI441

Mass Spectrometric Analysis of Monomolecular Layers of Solids by Secondary Ion Emission＆A．BENNINGHOVEN444

Mass Spectrometric Measurements of the Secondary Ion Emission of Alloys as an Analytical Tool＆V．CHEREPIN448

REACTION KINETICS,ETC．451

Mass Spectrometric Studies of Atomic and Free Radical Reactions＆JOHN T．HERRON453

Molecular Beam-Surface Interactions＆RICHARD P．BURNS and HOWARD L．BLAZ462

Development of a Time-of-Flight Mass Spectrometer to Monitor Fast Reactions＆S．E．APPLEBY,S．B．HOWARTH,P．HEALD,J．H．LIPPIATT,J．D．MADELEY,P．MYERS,W．J．ORVILLE-THOMAS,D．PRICE,AND G．B．WARD465

Kinetics by Mass Spectrometry:Molecular-Beam Sampling Applied to Pyrolysis of Hydrogen Peroxide＆A．TESSIER AND W．FORST471

Comparative Mass Spectrometric Study of the Same Heterogeneous Reaction in a Stationary Flow Reactor and a Molecular-Beam Apparatus＆R．DUCROS,H．G．LINTZ,A．PENTENERO,AND P．LE GOFF475

Direct Mass Spectrometric Measurements of the Rates of Association Reactions of Borane in the Gas Phase＆G．W．MAPPES,S．A．FRIDMANN,AND T．P．FEHLNER478

Contribution to Hot-Atom Reaction Studies:Formation of Organic Iodides in Solid Butane Irradiated by I+ Ions＆J．Ch．ABBE,J．M．PAULUS,J．CAILLERET,G．LAGARDE,J．MEYER,AND R．IGERSHEIM481

Mass Spectrometric Method for the Evaluation of Diffusion Characteristics of Rare Gases in Solids＆H．BAUR,U．FRICK,H．FUNK,L．SCHULTZ,AND P．SIGNER483

NEGATIVE IONS:MAGNETIC MOMENTS489

The Sampling of Negative Ion Populations in Townsend Discharges＆P．R．KINSMAN,J．MCGEEHAN,A．N．PRASAD,AND J．A．REES489

Ionization by Electron Impact of Some Inorganic Fluorides＆P．W．HARLAND AND J．C．J．THYNNE493

Mass Spectrometric Identification of the Paramagnetic Component of a Molecular beam＆V．L．TAL＇ROSE,A．F．DODONOV,I．O．LEIPUNSKII,AND I．I．MOROSOV497

Magnetic Moments of the Diatomic Molecules of the Transition Elements＆ERTHUR KANT AND FRANCIS MCCAFFREY500

APPLICATIONS TO SPACE STUDIES503

Mass Spectrometry Applied to Lunar Materials＆O．A．SCHAEFFER505

Upper Atmosphere Studies by Mass Spectrometry＆N．W．SPENCER509

Analysis of Lunar Materials by Spark-Source Mass Spectrometry＆G．H．MORRISON,A．T．KASHUBA,AND A．M．ROTHENBERG520

SPARK-SOURCE AND ANALYTICAL MASS SPECTROMETRY527

Improvements in Spark-Source Mass Spectrography Analysis by Use of Cryopumping＆FRANCIS BEGREVE529

Trace Analysis with the Matrix as Internal Standard＆A．M．ANDREANI,B．BLANCHARD,J．C．BRUN,J．P．MERMOUD,J．PELLET,AND R．STEFANI534

Analysis of Curium and Californium by Single-Exposure Spark-Source Mass Spectrometry＆P．CHASTAGNER AND B．TIFFANY539

Reactor Coolant Sodium Studies Using a Spark-Source Mass Spectrometer＆EDGAR BERKEY AND WILLIAM M．HICKAM543

Determination of Trace Amounts of Oxygen,Carbon,and Nitrogen in Metals by Spark-Source Mass Spectrography＆F．KONISHI AND N．NAKAMURA547

Continuous Analysis of Metallic Vapours by Mass Spectrometry＆PH．TYOU551

Dating of Geological Samples by K-Ar Method．Quantitative Dosing of the Three Isotopes of Argon by Mass Spectrometry＆H．BELLON AND J．Cl．PHILIPPET554

Applications of the Integrated Ion Current Technique to the Determination of Metal Chelates,Polycyclic Hydrocarbons,and Phenolic Amines,and to the Detection of Isomerism in Organic Compounds＆J．R．MAJER AND M．J．A．READE560

Mass Spectrometric Thermal Analysis of Organic Polymers＆HAROLD W．GOLDSTEIN563

ORGANIC COMPOUNDS567

Mass Spectrometry of Organic Compounds－a Review＆DUDLEY H．WILLIAMS569

Utilization of Mass Spectral Information for Molecular Structure Determination＆F．W．MCLAFFERTY589

The State and Future Development of GC-MS Methods and Techniques＆D．HENNEBERG AND G．SCHOMBURG605

Applications of a New Technique to the Analysis of GC Eluents＆M．BARBER,J．R．CHAPMAN,B．N．GREEN,AND T．O．MERREN615

Direct Coupling of a Gas Chromatographic Capillary Column and a Mass Spectrometer＆NICOLE SELLIER AND GEORGES GUIOCHON618

Polymerization of Organic Substances by High Electric Fields＆H．D．BECKEY,M．D．MIGAHED,AND F．W．ROLLGEN622

High- and Low-Resolution Field Desorption Mass Spectra of Organic Molecules＆H．D．BECKEY,G．HOFFMANN,K．H．MAURER,AND H．U．WINKLER626

The Use of Electron Attachment Mass Spectrography in the Analysis of Petroleum Hydrocarbons＆CZESLAW KAJDAS632

Ring Contraction in Molecular Ions of Acylated Alicyclic Amines as a Function of Ring Size＆W．J．RICHATER,J．M．TESAREK,AND A．L．BURLINGAME635

Electron-Impact Induced Fragmentation of ε-Diketones＆J．KOSSANYI639

Mass Spectrometry of Aralkyl Compounds with a Functional Group．Part XI:On the Symmetrization of the Molecular Ions from 2-Phenoxyethyl Halides＆C．B．THEISSLING,N．M．M．NIBBERING,AND TH．J．DE BOER642

The Fragmentation of Aminobenzophenones＆W．BENZ651

Intramolecular Substitution of Molecular Ions of Some Aromatic Compounds＆HANS-FRIEDRICH GRUTZMACHER,HEINZ KUSCHEL,AND PETER ADAMIETZ654

Localized Activation in Bond-Forming Reactions Under Electron Impact＆SEYMOUR MEYERSON AND L．C．LEITCH659

Ionization Study and Electronic Configurations of an Aliphatic Enones Family＆M．MONTAGNE,P．ARNAUD,P．NOUNOU,AND B．CABAUD662

Charge Location and Fragmentation under Electron Impact．III．Some Studies on Ethyl and Aryl Substituted Ureas and Related Compounds＆M．A．BALDWIN,P．C．CARDNELL,A．G．LOUDON,A．MACCOLL,AND K．S．WEBB666

The Investigation of a Transmission of Electronic Influences Through the Chain of Conjugated Double Bonds by Mass Spectrometry＆B．M．ZOLOTAREV,L．A．YANOWSKAYA,B．UMIRZAKOV,O．S．CHIZHOV,AND V．F．KUCHEROV670

Stereospecific Fragmentation of Isomeric Diesters＆A．MANDELBAUM,J．DEUTSCH,A．KARPATI,AND I．MERKSAMMER672

The Mass Spectra of Some bis-Aziridinones:Consecutive Loss of Two CO Molecules from Separate Rings＆ISTVAN LENGYEL,DAVID B．ULISS,AND ROBERT V．MARK676

Mass Spectrometry of Unsaturated Alcohols＆DAVID G．I．KINGSTON AND HARVEY P．TANNENBAUM681

New Fragmentation Reactions Observed in the Mass Spectra of Macrocyclic Spermidine Alkaloids＆H．J．VEITH AND M．HESSE685

Some Stereospecific Fragmentations in the Mass Spectra of Steroids＆HANS-WOLFRAM FEHLHABER,DIETER LENOIR,AND PETER WELZEL689

The Influence of the Central Metal Atom on the Fragmentation of Chromium-π-complexes＆J．MULLER AND K．FENDERL693

Mass Spectrometric Study of Transition Metal Complexes with Ligands Having Nitrogen or Sulphur as Donor Atom＆G．DISTEFANO,A．FOFFANI,G．INNORTA AND S．PIGNATARO696

Determination of Bond Energies of Organic Silicon Compounds on the Basis of Appearance Potentials＆J．BOROSSAY AND L．SZEPES700

Mass Spectrometric Examination of Methoxy- and Ethoxy-Methylsilanes＆J．TAMAS,K．UJSZASZY,AND GY．BUJTAS703

Ion Structures in Norbornyl Compounds＆J．L．HOLMES AND D．MCGILLIVRAY706

Pyrolytic and Electron-Impact Reactions of Cyclic Sulphites and Carbonates of Aromatic Diols＆DON C．DEJONGH709

BIOCHEMICAL APPLICATIONS713

The Role of Mass Spectrometry in Biochemistry and Related Fields＆JAMES A．MCCLOSKEY715

A Quantitative Approach to Protein Sequencing Using Mass Spectrometry＆C．PERRINE,E．CANNON,C．CAVENDER,T．FAIRWELL,AND R．E．LOVINS728

Application of the Method of Photo-ionization to Mass Spectrometric Determination of Amino Acid Sequence in Short Peptides＆JA．M．VARSHAVSKY AND V．M．ORLOV735

Mass Spectrometry of Bile Pigments Structure of Phycocyanobilin＆B．L．SCHRAM738

The Quantitative High-Resolution Mass Spectrometry of Human Tissue Volatiles:the Determination of Certain Purines and Purine Analogues in the Skeletal Muscle of Gout Patients＆W．SNEDDEN,R．B．PARKER,AND R．W．E．WATTS742

Determination fo 18O in Compounds Isolated from Bacteria Growth on 18O Labelled Hexoses＆R．B．JOHNSON,L．PONTICORVO,AND D．RITTENBERG746

Quantitative Determination of Trace Metals by Electron Impact Ionization Mass Spectrometry＆J．K．TERLOUW AND G．DIJKSTRA748

High-Resolution Mass Spectrometry of Ribonucleic Acid Hydrolysates＆A．M．LAWSON,W．A．KOENIG,L．C．SMITH,N．R．EARLE,AND JAMES A．MCCLOSKEY753

Sequence Analysis of Tri- and Tetranucleotides by Mass Spectrometry＆J．L．WIEBERS757

Mass Spectrometric Sequence Determination of Permethylated Methionine-Containing Peptides＆P．ROEPSTORFF,K．NORRIS,S．SEVERINSEN,AND K．BRUNFELDT761